Not really. If you ask me, they're Slug-Toad-Snake deadlock is also found in their accomplishments. Jiraiya was able to achieve wealth while Tsunade constantly lost money due to gambling. He also achieved Sage Mode, whilst Orochimaru did not.
Tsunade became Hokage while Orochimaru failed to do so.
Tsunade's medical ninjutsu is unable to raise the dead, as she would have wanted for Dan and Nawaki, while Orochimaru can do so with Edo Tensei.
Jiraiya wanted to achieve peace, and was unable to do so. On the other hand, Orochimaru's help resulted in major help for the protagonists in the Fourth Shinobi World, without which true peace would not have been achieved.